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Salinity exchange between seawater/brackish water and domestic wastewater through electrodialysis forpotable water

《环境科学与工程前沿(英文)》 2023年 第17卷 第2期 doi: 10.1007/s11783-023-1616-1

摘要:

● Present a general concept called “salinity exchange”.

关键词: Desalination     Potable water reuse     Ion-exchange membrane     Salinity gradient energy     Wastewater discharge    

The energy-free purification of trace thallium(I)-contaminated potable water using a high-selective filter

《化学科学与工程前沿(英文)》 doi: 10.1007/s11705-023-2379-8

摘要: Thallium is a highly toxic metal, and trace amount of thallium(I) (Tl+) in potable water could cause a severe water crisis, which arouses the exploitation of highly-effective technology for purification of Tl+ contaminated water. This report proposes the multi-layered Prussian blue (PB)-decorated composite membranes (PBx@PDA/PEI-FP) based on the aminated filter papers for Tl+ uptake. Extensively characterization by Fourier transform infrared spectrometer-attenuated total reflectance, scanning electron microscope, thermogravimetric analysis, X-ray photoelectron spectroscopy and X-ray diffraction were performed to confirm the in situ growth of cubic PB crystals on filter paper membrane surfaces via the aminated layers, and the successful fabrication of multi-layered PB overcoats via the increasing of aminated layers. The effect of PB layers on Tl+ removal by PBx@PDA/PEI-FP from simulated drinking water was evaluated as well as the influence of different experimental conditions. A trade-off between PB decoration layer number and PB distribution sizes is existed in Tl+ uptake by PBx@PDA/PEI-FP. The double-layered PB2@PDA/PEI-FP membrane showed the maximum sorption capacity, but its Tl+ uptake performance was weakened by the acid, coexisting ions (K+ and Na+) and powerful operation pressure, during filtrating a large volume of low-concentrated Tl+-containing water. However, the negative effect of coexisting ions on the Tl+ uptake could be effectively eliminated in weak alkaline water, and the Tl+ removal was increased up to 100% without any pressure driving for PB2@PDA/PEI-FP membrane. Most importantly, PB2@PDA/PEI-FP displayed the high-efficiency and high-selectivity in purifying the Tl+-spiked Pearl River water, in which the residual Tl+ in filtrate was less than 2 μg·L–1 to meet the drinking water standard of United States Environmental Protection Agency. This work provides a feasible avenue to safeguard the drinking water in remote and underdeveloped area via the energy-free operation.

关键词: membrane adsorption     Prussian blue     energy-free filtration     potable water     trace thallium(I)    

膜技术在饮用水深度处理中的应用现状

吴礼光,赵海洋,张林

《中国工程科学》 2014年 第16卷 第7期   页码 106-112

摘要:

从压力驱动膜及膜集成技术的特点出发,结合不同水源水质,对膜技术应用于饮用水深度处理方面的进展进行了分析和综述,并提出膜法饮用水深度处理的发展建议。

关键词: 膜技术     集成过程     饮用水深度处理    

Role of water chemistry on estrone removal by nanofiltration with the presence of hydrophobic acids

Xue JIN,Jiangyong HU

《环境科学与工程前沿(英文)》 2015年 第9卷 第1期   页码 164-170 doi: 10.1007/s11783-014-0747-9

摘要: Hydrophobic acid organic matter (HpoA) extracted from treated effluent has been known to improve the rejection of steroid hormone estrone by reverse osmosis (RO) and nanofiltration (NF) membranes. In this study, the effects of solution chemistry (solution pH and ionic strength) on the estrone rejection by NF membrane with the presence of HpoA were systematically investigated. Crossflow nanofiltration experiments show that the presence of HpoA significantly improved estrone rejection at all pH and ionic strength levels investigated. It is consistently shown that the “enhancement effect” of HpoA on estrone rejection at neutral and alkaline pH is attributed to the binding of estrone by HpoA macromolecules via hydrogen bonding between phenolic functional groups in feed solutions, which leads to an increase in molecular weight and appearance of negative charge. The membrane exhibited the best performance in terms of estrone rejection at pH 10.4 (compared to pH 4 and pH 7) as a result of strengthening the electrostatic repulsion between estrone and membrane with the presence of HpoA. At neutral pH level, the ability of HpoA macromolecules to promote estrone rejection became stronger with increasing ionic strength due to their more extended conformation, which created more chances for the association between estrone and HpoA. The important conclusion of this study is that increasing solution pH and salinity can greatly intensify the “enhancement effect” of HpoA. These results can be important for NF application in direct/indirect potable water reuse.

关键词: indirect potable water reuse     steroid hormone     nanofiltration(NF)     rejection     water chemistry     hydrophobic acids    

水·水资源·农业节水

刘更另

《中国工程科学》 2000年 第2卷 第7期   页码 39-42

摘要:

文章从水性质特点谈到中国水资源的问题,认为不能单纯用年平均降雨量的多少来判定中国水资源的状况,水资源开发利用的好坏决定于人类社会的调节和管理。中国水资源总的来说是够用的,最大问题是降水量的时空分布不平衡。

中国农民几千年来创造了许多治水蓄水用水的经验。农业节水非常重要,关键在"分散蓄水,分散使用",以减少径流在汇集和分散过程中的损失和污染,在提高水的利用效率方面有一系列的科研和实际工作要做。

关键词:     水资源     农业节水     分散蓄水    

Managing water for life

Daniel P. LOUCKS, Haifeng JIA

《环境科学与工程前沿(英文)》 2012年 第6卷 第2期   页码 255-264 doi: 10.1007/s11783-011-0359-6

摘要: Water is essential for life. In spite of the entire engineering infrastructure devoted to the treatment, regulation and beneficial uses of water, occasionally sufficient quantities and qualities of water become scarce. When this happens, just how do we decide how much less water to allocate to all of us and the activities we engage in to sustain and enhance our quality of life? This paper addresses some of the complexities of answering such a question, especially as society increasingly recognizes the need to provide flow regimes that will maintain healthy aquatic and floodplain ecosystems that also impact the economic, physical and even the spiritual quality of our lives. For we depend on these ecosystems to sustain our wellbeing. We are indeed a part of our ecosystems. We depend upon on aquatic ecosystems to moderate river flow qualities and quantities, reduce the extremes of floods and droughts, reduce erosion, detoxify and decompose waterborne wastes, generate and preserve flood plain soils and renew their fertility, regulate disease carrying organisms, and to enhance recreational benefits of river systems. This question of deciding just how much water to allocate to each water user and for the maintenance of viable aquatic ecosystems, especially when there is not enough, is a complex, and largely political, issue. This issue is likely to become even more complex and political and contentious in the future as populations grow and as water quantities and their qualities become even more variable and uncertain.

关键词: water stress     aquatic ecosystems     sustainable water resource allocations     ecosystem water requirements    

The effect of different agricultural management practices on irrigation efficiency, water use efficiencyand green and blue water footprint

La ZHUO, Arjen Y. HOEKSTRA

《农业科学与工程前沿(英文)》 2017年 第4卷 第2期   页码 185-194 doi: 10.15302/J-FASE-2017149

摘要: This paper explores the effect of varying agricultural management practices on different water efficiency indicators: irrigation efficiency (IE), crop water use efficiency (WUE), and green and blue water footprint (WF). We take winter wheat in an experimental field in Northern China as a case study and consider a dry, average and wet year. We conducted 24 modeling experiments with the AquaCrop model, for all possible combinations of four irrigation techniques, two irrigation strategies and three mulching methods. Results show that deficit irrigation most effectively improved blue water use, by increasing IE (by 5%) and reducing blue WF (by 38%), however with an average 9% yield reduction. Organic or synthetic mulching practices improved WUE (by 4% and 10%, respectively) and reduced blue WF (by 8% and 17%, respectively), with the same yield level. Drip and subsurface drip irrigation improved IE and WUE, but drip irrigation had a relatively large blue WF. Improvements in one water efficiency indicator may cause a decline in another. In particular, WUE can be improved by more irrigation at the cost of the blue WF. Furthermore, increasing IE, for instance by installing drip irrigation, does not necessarily reduce the blue WF.

关键词: field management     irrigation efficiency     water footprint     water productivity     water use efficiency    

Emergency drinking water treatment in source water pollution incident-technology and practice in China

Xiaojian ZHANG , Chao CHEN ,

《环境科学与工程前沿(英文)》 2009年 第3卷 第3期   页码 364-368 doi: 10.1007/s11783-009-0027-2

摘要: An investigation into emergency potable water treatment technologies was conducted to investigate China’s water pollution situation. In order to confirm optimum parameters, the technological efficiency of each pollutant was obtained. About 100 contaminants were tested to find the emergency treatment technologies, most of which were found to be positive. This paper presents the three largest and most significant water pollution incidents in China to date, analyzing cases such as the nitrobenzene pollution incident in the Songhua River in November 2005, the cadmium pollution incident in the Beijiang River in December 2005, and the water crisis with odorous tap water in Wuxi City in May 2007.

关键词: emergency drinking water treatment     water pollution     adsorption     oxidation     precipitation    

Molecular analysis of bacterial community in the tap water with different water ages of a drinking water

Feng Wang, Weiying Li, Yue Li, Junpeng Zhang, Jiping Chen, Wei Zhang, Xuan Wu

《环境科学与工程前沿(英文)》 2018年 第12卷 第3期 doi: 10.1007/s11783-018-1020-4

摘要: Bacterial community in the drinking water distribution system (DWDS) was regulated by multiple environmental factors, many of which varied as a function of water age. In this study, four water samples with different water ages, including finished water (FW, 0 d) and tap water (TW) [TW1 (1 d), TW2(2 d) and TW3(3 d)], were collected along with the mains of a practical DWDS, and the bacterial community was investigated by high-throughput sequencing technique. Results indicated that the residual chlorine declined with the increase of water age, accompanied by the increase of dissolved organic matter, total bacteria counts and bacterial diversity (Shannon). For bacterial community composition, although Proteobacteria phylum (84.12%-97.6%) and Alphaproteobacteria class (67.42%-93.09%) kept dominate, an evident regular was observed at the order level. In detail, the relative abundance of most of other residual orders increased with different degrees from the start to the end of the DWDS, while a downward trend was uniquely observed in terms of Rhizobiales, who was inferred to be chlorine-resistant and be helpful for inhibiting pipes corrosion. Moreover, some OTUs were found to be closely related with species possessing pathogenicity and chlorine-resistant ability, so it was recommended that the use of agents other than chlorine or agents that can act synergically with chlorine should be developed for drinking water disinfection. This paper revealed bacterial community variations along the mains of the DWDS and the result was helpful for understanding bacterial ecology in the DWDS.

关键词: Bacterial community     Water age     High-throughput sequencing technique     Drinking water distribution system    

Comparative genotoxicity of water processed by three drinking water treatment plants with different water

Ting Zhang, Heze Liu, Yiyuan Zhang, Wenjun Sun, Xiuwei Ao

《环境科学与工程前沿(英文)》 2020年 第14卷 第3期 doi: 10.1007/s11783-020-1214-4

摘要: Genotoxicity of substances is unknown in the water after treatment processes. Genotoxicity decreased by activated carbon treatment but increased by chlorination. Halogenated hydrocarbons and aromatic compounds contribute to genotoxicity. Genotoxicity was assessed by umu test; acute and chronic toxicity by ECOSAR. Inconsistent results confirmed that genotoxicity cannot be assessed by ECOSAR. Advanced water treatment is commonly used to remove micropollutants such as pesticides, endocrine disrupting chemicals, and disinfection byproducts in modern drinking water treatment plants. However, little attention has been paid to the changes in the genotoxicity of substances remaining in the water following the different water treatment processes. In this study, samples were collected from three drinking water treatment plants with different treatment processes. The treated water from each process was analyzed and compared for genotoxicity and the formation of organic compounds. The genotoxicity was evaluated by an umu test, and the acute and chronic toxicity was analyzed through Ecological Structure- Activity Relationship (ECOSAR). The results of the umu test indicated that biological activated carbon reduced the genotoxicity by 38%, 77%, and 46% in the three drinking water treatment plants, respectively, while chlorination increased the genotoxicity. Gas chromatograph-mass spectrometry analysis revealed that halogenated hydrocarbons and aromatic compounds were major contributors to genotoxicity. The results of ECOSAR were not consistent with those of the umu test. Therefore, we conclude that genotoxicity cannot be determined using ECOSAR .

关键词: Drinking water     Treatment process     Genotoxicity     Umu test     Ecological Structure-Activity Relationship    

Bioinspired and biomimetic membranes for water purification and chemical separation: A review

《环境科学与工程前沿(英文)》 2021年 第15卷 第6期 doi: 10.1007/s11783-021-1412-8

摘要:

•The history of biological and artificial water channels is reviewed.

关键词: Aquaporins     Artificial water channels     Biomimetic membranes     Chemical separation and water purification    

A red water occurrence in drinking water distribution systems caused by changes in water source in Beijing

ZHANG Xiaojian,MI Zilong,WANG Yang,LIU Shuming,NIU Zhangbin,LU Pinpin,WANG Jun,GU Junnong,CHEN Chao

《环境科学与工程前沿(英文)》 2014年 第8卷 第3期   页码 417-426 doi: 10.1007/s11783-013-0558-4

摘要: A red water phenomenon occurred in several communities few days after the change of water source in Beijing, China in 2008. In this study, the origin of this problem, the mechanism of iron release and various control measures were investigated. The results indicated that a significant increase in sulphate concentration as a result of the new water source was the cause of the red water phenomenon. The mechanism of iron release was found that the high-concentration sulphate in the new water source disrupted the stable shell of scale on the inner pipe and led to the release of iron compounds. Experiments showed that the iron release rate in the new source water within pipe section was over 11-fold higher than that occurring within the local source water. The recovery of tap water quality lasted several months despite ameliorative measures being implemented, including adding phosphate, reducing the overall proportion of the new water source, elevating the pH and alkalinity, and utilizing free chlorine as a disinfectant instead of chloramine. Adding phosphate was more effective and more practical than the other measures. The iron release rate was decreased after the addition of 1.5 mg·L orthophosphate- P, tripolyphosphate-P and hexametaphosphate-P by 68%, 83% and 87%, respectively. Elevating the pH and alkalinity also reduced the iron release rate by 50%. However, the iron release rate did not decreased after replacing chloramine by 0.5–0.8 mg·L of free chlorine as disinfectant.

关键词: iron release     drinking water distribution system     sulphate     phosphate     red water control     water quality stability    

Water, energy and food interactions–Challenges and opportunities

Gustaf OLSSON

《环境科学与工程前沿(英文)》 2013年 第7卷 第5期   页码 787-793 doi: 10.1007/s11783-013-0526-z

摘要: Water and energy are inextricably linked, and as a consequence both have to be addressed together. This is called the water-energy nexus. When access to either is limited, it becomes obvious that it is necessary to consider their interdependence. Population growth, climate change, urbanization, increasing living standards and food consumption will require an integrated approach where food, water and energy security are considered together. In this paper we examine water, energy and food security and their couplings. The nexus also creates conflicts between water use, energy extraction and generation as well as food production. Some of these conflicts are illustrated. It is argued that there is an urgent need for integrated planning and operation. Not only will better technology be needed, but also better integration of policies, organizations and political decisions.

关键词: water security     energy security     food security     water-energy nexus     water conflicts    

标题 作者 时间 类型 操作

Salinity exchange between seawater/brackish water and domestic wastewater through electrodialysis forpotable water

期刊论文

The energy-free purification of trace thallium(I)-contaminated potable water using a high-selective filter

期刊论文

膜技术在饮用水深度处理中的应用现状

吴礼光,赵海洋,张林

期刊论文

Role of water chemistry on estrone removal by nanofiltration with the presence of hydrophobic acids

Xue JIN,Jiangyong HU

期刊论文

巨晓洁:用于水处理和水检测的新型功能材料(2022年4月16日)

2022年06月09日

会议视频

水·水资源·农业节水

刘更另

期刊论文

王光谦:全球水循环与水资源利用(2019年10月17日)

王光谦(院士)

2021年01月20日

会议视频

Managing water for life

Daniel P. LOUCKS, Haifeng JIA

期刊论文

The effect of different agricultural management practices on irrigation efficiency, water use efficiencyand green and blue water footprint

La ZHUO, Arjen Y. HOEKSTRA

期刊论文

Emergency drinking water treatment in source water pollution incident-technology and practice in China

Xiaojian ZHANG , Chao CHEN ,

期刊论文

Molecular analysis of bacterial community in the tap water with different water ages of a drinking water

Feng Wang, Weiying Li, Yue Li, Junpeng Zhang, Jiping Chen, Wei Zhang, Xuan Wu

期刊论文

Comparative genotoxicity of water processed by three drinking water treatment plants with different water

Ting Zhang, Heze Liu, Yiyuan Zhang, Wenjun Sun, Xiuwei Ao

期刊论文

Bioinspired and biomimetic membranes for water purification and chemical separation: A review

期刊论文

A red water occurrence in drinking water distribution systems caused by changes in water source in Beijing

ZHANG Xiaojian,MI Zilong,WANG Yang,LIU Shuming,NIU Zhangbin,LU Pinpin,WANG Jun,GU Junnong,CHEN Chao

期刊论文

Water, energy and food interactions–Challenges and opportunities

Gustaf OLSSON

期刊论文